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- 01GPJRY85QPH03DGKH4NJYNGAC classification A1.
- 01GPJRY85QPH03DGKH4NJYNGAC date "2022".
- 01GPJRY85QPH03DGKH4NJYNGAC language "eng".
- 01GPJRY85QPH03DGKH4NJYNGAC type journalArticle.
- 01GPJRY85QPH03DGKH4NJYNGAC hasPart 01GPJSTX61JYGM72JKH8MJ9STA.pdf.
- 01GPJRY85QPH03DGKH4NJYNGAC hasPart urn:uuid:084fa76a-a0a5-405f-b7ed-1fdabeb4fd11.
- 01GPJRY85QPH03DGKH4NJYNGAC hasPart urn:uuid:c0784da1-a1d3-4566-bbf6-8322a6686f2b.
- 01GPJRY85QPH03DGKH4NJYNGAC subject "Chemistry".
- 01GPJRY85QPH03DGKH4NJYNGAC subject "Physics and Astronomy".
- 01GPJRY85QPH03DGKH4NJYNGAC doi "10.1016/j.xcrp.2022.100874".
- 01GPJRY85QPH03DGKH4NJYNGAC issn "2666-3864".
- 01GPJRY85QPH03DGKH4NJYNGAC issue "5".
- 01GPJRY85QPH03DGKH4NJYNGAC volume "3".
- 01GPJRY85QPH03DGKH4NJYNGAC abstract "Artificial photosynthesis of H2O2, an environmentally friendly oxidant and a clean fuel, holds great promise. However, improving its efficiency and stability for industrial implementation remains highly challenging. Here, we report the visible-light H2O2 artificial photosynthesis by digging pro-superoxide radical carbon vacancies in three-dimensional hierarchical porous g-C3N4 through a simple hydrolysis-freeze-drying-thermal treatment. A significant electronic structure change is revealed upon the implantation of carbon vacancies, broadening visible-light absorption and facilitating the photogenerated charge separation. The strong electron affinity of the carbon vacancies promotes superoxide radical (O-center dot(2)-) formation, significantly boosting the H2O2 photocatalytic production. The developed photocatalyst shows an H2O2 evolution rate of 6287.5 mM g(-1) h(-1) under visible-light irradiation with a long cycling stability being the best-performing photocatalyst among all reported g-C3N4-based systems. Our work provides fundamental insight into highly active and stable photocatalysts with great potential for safe industrial H2O2 production.".
- 01GPJRY85QPH03DGKH4NJYNGAC author F503F252-F0ED-11E1-A9DE-61C894A0A6B4.
- 01GPJRY85QPH03DGKH4NJYNGAC author urn:uuid:2a9f15ea-12d7-413b-b725-416e34ded552.
- 01GPJRY85QPH03DGKH4NJYNGAC author urn:uuid:59bc0d80-d23e-4187-8570-85f3adfaf347.
- 01GPJRY85QPH03DGKH4NJYNGAC author urn:uuid:6fc20fa6-8be5-4b8f-bae9-cc551c454c1c.
- 01GPJRY85QPH03DGKH4NJYNGAC author urn:uuid:7ddbe5d3-597a-475a-a4b1-29a6d3183493.
- 01GPJRY85QPH03DGKH4NJYNGAC author urn:uuid:9c4672e4-31fd-43fb-8719-c9fce1b719d2.
- 01GPJRY85QPH03DGKH4NJYNGAC author urn:uuid:a6c63c5d-9f10-48ec-9ee7-a27b2f219f2b.
- 01GPJRY85QPH03DGKH4NJYNGAC author urn:uuid:b2342f1b-1c90-4fc5-980e-03da70a3c098.
- 01GPJRY85QPH03DGKH4NJYNGAC author urn:uuid:b2ff84a2-a601-425a-8917-008b336dd48a.
- 01GPJRY85QPH03DGKH4NJYNGAC author urn:uuid:b7f71816-c675-400b-81c3-c124b2c5ef22.
- 01GPJRY85QPH03DGKH4NJYNGAC author urn:uuid:e6d1ec84-da34-4da0-91d8-584354379054.
- 01GPJRY85QPH03DGKH4NJYNGAC author urn:uuid:f9caf6c0-a17b-4c4a-97ae-e757ddc4cf5c.
- 01GPJRY85QPH03DGKH4NJYNGAC dateCreated "2023-01-12T10:38:18Z".
- 01GPJRY85QPH03DGKH4NJYNGAC dateModified "2025-01-28T09:36:10Z".
- 01GPJRY85QPH03DGKH4NJYNGAC name "Photochemical production of hydrogen peroxide by digging pro-superoxide radical carbon vacancies in porous carbon nitride".
- 01GPJRY85QPH03DGKH4NJYNGAC pagination urn:uuid:5402953e-2201-415a-a749-5dfdaed5ac72.
- 01GPJRY85QPH03DGKH4NJYNGAC sameAs LU-01GPJRY85QPH03DGKH4NJYNGAC.
- 01GPJRY85QPH03DGKH4NJYNGAC sourceOrganization urn:uuid:7cfa214f-5d30-4d9d-a102-fcd4f90221f1.
- 01GPJRY85QPH03DGKH4NJYNGAC type A1.