Matches in Ghent University Academic Bibliography for { <https://biblio.ugent.be/publication/01J15B7JSP5MQV0CZ1FH5CSDG8> ?p ?o. }
Showing items 1 to 25 of
25
with 100 items per page.
- 01J15B7JSP5MQV0CZ1FH5CSDG8 classification A1.
- 01J15B7JSP5MQV0CZ1FH5CSDG8 date "2024".
- 01J15B7JSP5MQV0CZ1FH5CSDG8 language "eng".
- 01J15B7JSP5MQV0CZ1FH5CSDG8 type journalArticle.
- 01J15B7JSP5MQV0CZ1FH5CSDG8 hasPart 01J15BS8JGEPR7Y99ZPK1441GZ.pdf.
- 01J15B7JSP5MQV0CZ1FH5CSDG8 subject "Chemistry".
- 01J15B7JSP5MQV0CZ1FH5CSDG8 subject "Physics and Astronomy".
- 01J15B7JSP5MQV0CZ1FH5CSDG8 doi "10.1002/smll.202307090".
- 01J15B7JSP5MQV0CZ1FH5CSDG8 issn "1613-6810".
- 01J15B7JSP5MQV0CZ1FH5CSDG8 issn "1613-6829".
- 01J15B7JSP5MQV0CZ1FH5CSDG8 issue "22".
- 01J15B7JSP5MQV0CZ1FH5CSDG8 volume "20".
- 01J15B7JSP5MQV0CZ1FH5CSDG8 abstract "The use of functional materials is a popular strategy to mitigate the polysulfide-induced accelerated aging of lithium-sulfur (Li-S) batteries. However, deep insights into the role of electrode design and formulation are less elaborated in the available literature. Such information is not easy to unearth from the existing reports on account of the scattered nature of the data and the big dissimilarities among the reported materials, preparation protocols, and cycling conditions. In this study, model functional materials known for their affinity toward polysulfide species, are integrated into the porous sulfur electrodes at different quantities and with various spatial distributions. The electrodes are assembled in 240 lithium-sulfur cells and thoroughly analyzed for their short- and long-term electrochemical performance. Advanced data processing and visualization techniques enable the unraveling of the impact of porous electrodes' formulation and design on self-discharge, sulfur utilization, and capacity loss. The results highlight and quantify the sensitivity of the cell performance to the synergistic interactions of catalyst loading and its spatial positioning with respect to the sulfur particles and carbon-binder domain. The findings of this work pave the road for a holistic optimization of the advanced sulfur electrodes for durable Li-S batteries. This research seeks to offer key insights into optimizing advanced electrodes for lithium-sulfur batteries. The study emphasizes the critical role of optimal catalyst quantity and strategic placement near sulfur particles or the carbon-binder domain. These factors notably impact capacity retention and rate-capability, governing the local balance between the conversion and migration rates of polysulfides.image".
- 01J15B7JSP5MQV0CZ1FH5CSDG8 author 1DFA8BB4-F59C-11E1-8C35-769E10BDE39D.
- 01J15B7JSP5MQV0CZ1FH5CSDG8 author F552BC16-F0ED-11E1-A9DE-61C894A0A6B4.
- 01J15B7JSP5MQV0CZ1FH5CSDG8 author urn:uuid:915187f5-2293-4f83-a89d-0f034acf9483.
- 01J15B7JSP5MQV0CZ1FH5CSDG8 author urn:uuid:a1257bdb-1a9b-47a0-96b8-797088596df8.
- 01J15B7JSP5MQV0CZ1FH5CSDG8 author urn:uuid:bc2489ca-706d-412d-bb5f-a3ced53f5816.
- 01J15B7JSP5MQV0CZ1FH5CSDG8 dateCreated "2024-06-24T14:43:35Z".
- 01J15B7JSP5MQV0CZ1FH5CSDG8 dateModified "2024-12-12T21:14:15Z".
- 01J15B7JSP5MQV0CZ1FH5CSDG8 name "Toward a synergistic optimization of porous electrode formulation and polysulfide regulation in lithium-sulfur batteries".
- 01J15B7JSP5MQV0CZ1FH5CSDG8 pagination urn:uuid:e1cba263-8712-4622-a7e6-e5214f8119a1.
- 01J15B7JSP5MQV0CZ1FH5CSDG8 sameAs LU-01J15B7JSP5MQV0CZ1FH5CSDG8.
- 01J15B7JSP5MQV0CZ1FH5CSDG8 sourceOrganization urn:uuid:7b187b24-9f58-42c4-8cc6-7f6c3bf1a333.
- 01J15B7JSP5MQV0CZ1FH5CSDG8 type A1.