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- aggregation classification "C3".
- aggregation creator person.
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- aggregation date "2010".
- aggregation format "application/pdf".
- aggregation hasFormat 1077541.bibtex.
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- aggregation language "eng".
- aggregation rights "I have retained and own the full copyright for this publication".
- aggregation subject "Chemistry".
- aggregation title "A detailed study of the catalytic performance of V, Co and Cu MOFs in the oxidation of cyclohexene".
- aggregation abstract "In this research, the catalytic performance of V-, Co- and Cu-MOFs, prepared with 1,4-benzenedicarboxylic (BDC) and/or 1,3,5-benzenetricarboxylic (BTC) ligands, is discussed for the oxidation of cyclohexene. Several parameters have been examined, for example: solvent, temperature and oxidans. The detailed product distributions and recyclability of these materials are discussed. Surprisingly, the highest conversions and highest yields of epoxide are achieved with the coordinatively saturared V-MOF, MIL-47. Indeed, these MOFs have a completely different geometry and coordination of the metal centre, which will be discussed in relation to the catalytic results. The Cu-MOFs studied have a Cu2 or Co2 paddle-wheel structure in which the metal centres have a square coordination to bidentate carboxylate ligands. The latter can be unsaturated (activated CuBTC and CuBDC) or saturated (CoBDC-DABCO). The studied V-MOF, MIL-47, has a three-dimensional orthorhombic structure in which every V centre is completely saturated [1].".
- aggregation authorList BK103497.
- aggregation endPage "266".
- aggregation startPage "266".
- aggregation aggregates 1077545.
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