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- aggregation classification "A1".
- aggregation creator person.
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- aggregation date "2012".
- aggregation format "application/pdf".
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- aggregation isPartOf urn:issn:1751-7907.
- aggregation language "eng".
- aggregation rights "I have retained and own the full copyright for this publication".
- aggregation subject "Earth and Environmental Sciences".
- aggregation title "Catalytic dechlorination of diclofenac by biogenic palladium in a microbial electrolysis cell".
- aggregation abstract "Diclofenac is one of the most commonly detected pharmaceuticals in wastewater treatment plant (WWTP) effluents and the receiving water bodies. In this study, biogenic Pd nanoparticles (bio-Pd) were successfully applied in a microbial electrolysis cell (MEC) for the catalytic reduction of diclofenac. Hydrogen gas was produced in the cathodic compartment, and consumed as a hydrogen donor by the bio-Pd on the graphite electrodes. In this way, complete dechlorination of 1 mg diclofenac l-1 was achieved during batch recirculation experiments, whereas no significant removal was observed in the absence of the biocatalyst. The complete dechlorination of diclofenac was demonstrated by the concomitant production of 2-anilinophenylacetate (APA). Through the addition of -0.8 V to the circuit, continuous and complete removal of diclofenac was achieved in synthetic medium at a minimal HRT of 2 h. Continuous treatment of hospital WWTP effluent containing 1.28 mu g diclofenac l-1 resulted in a lower removal efficiency of 57%, which can probably be attributed to the affinity of other environmental constituents for the bio-Pd catalyst. Nevertheless, reductive catalysis coupled to sustainable hydrogen production in a MEC offers potential to lower the release of micropollutants from point-sources such as hospital WWTPs.".
- aggregation authorList BK489628.
- aggregation endPage "402".
- aggregation issue "3".
- aggregation startPage "396".
- aggregation volume "5".
- aggregation aggregates 4398659.
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- aggregation similarTo j.1751-7915.2011.00325.x.
- aggregation similarTo LU-2108767.