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- aggregation classification "A1".
- aggregation creator B169681.
- aggregation creator person.
- aggregation creator person.
- aggregation creator person.
- aggregation date "2014".
- aggregation format "application/pdf".
- aggregation hasFormat 5743578.bibtex.
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- aggregation isPartOf urn:issn:1759-9954.
- aggregation language "eng".
- aggregation rights "I have transferred the copyright for this publication to the publisher".
- aggregation subject "Chemistry".
- aggregation title "Synthesis of multi-functionalized hydrogels by a thiolactone-based synthetic protocol".
- aggregation abstract "We established a simplified synthetic protocol for the preparation of multiple functionalized hydrogels, which is potentially employable for the fabrication of adaptable sensors, using the recently introduced thiolactone chemistry. Thiolactone groups can be opened with a primary amine, through which a functional group is introduced, while at the same time a thiol is released, which is available for crosslinking or further functionalization. In this respect, a thiolactone functionalized poly(N-isopropylacryl amide) (p(NIPAAm-co-TlaAm)) precursor, obtained via RAFT, and 3-morpholinopropylamine or histamine as the ring opening amines are used to synthesize gels responding to CO2. The synthetic protocol relies on a newly discovered crosslinking mechanism involving the solvent dichloromethane as the crosslinking agent. We discuss the gel formation protocol in detail, including the crosslinking mechanism, and additionally demonstrate the response of the synthesized gels towards CO2. Finally, we show how the applied synthetic protocol can be used for the preparation of multiple functionalized gels, extending the concept to optical response type gels.".
- aggregation authorList BK418280.
- aggregation endPage "5470".
- aggregation issue "18".
- aggregation startPage "5461".
- aggregation volume "5".
- aggregation aggregates 5743584.
- aggregation isDescribedBy 5743578.
- aggregation similarTo c4py00468j.
- aggregation similarTo LU-5743578.